Recognition of copper and hydrogen sulfide in vitro using a fluorescein derivative indicator

Dalton Trans. 2012 May 21;41(19):5799-804. doi: 10.1039/c2dt12462a. Epub 2012 Mar 22.

Abstract

We report the development of a fluorescein-based chemosensor (L1) for monitoring ions or micromolecules (H(2)S). Copper ions are known to be toxic at high concentrations and hydrogen sulfide induces various problems. Herein we develop a simple method for detecting Cu(II) and H(2)S with high selectivity and sensitivity. The chemosensor L1 displays on-off-on type fluorescence change with alternately added Cu(II) and H(2)S to the media along with reversible forming-separating of the complex. The potential biomedical relevance of the chemical mechanisms involved in the detection of L1 is described.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Copper / analysis*
  • Copper / chemistry
  • Crystallography, X-Ray
  • Fluorescein / analysis
  • Fluorescein / chemistry*
  • Fluorescent Dyes / analysis
  • Fluorescent Dyes / chemistry*
  • Hep G2 Cells
  • Humans
  • Hydrogen Sulfide / analysis*
  • Hydrogen Sulfide / chemistry
  • Mice
  • Models, Molecular
  • Molecular Conformation
  • Molecular Imaging

Substances

  • Fluorescent Dyes
  • Copper
  • Fluorescein
  • Hydrogen Sulfide