Effects of Ce on catalytic combustion of methane over Pd-Pt/Al2O3 catalyst

J Environ Sci (China). 2012;24(3):507-11. doi: 10.1016/s1001-0742(11)60798-5.

Abstract

Activity and stability of 1%Pd-0.2%Pt/Al2O3 and 1%Pd-0.2%Pt/0.6%Ce/Al2O3 catalysts prepared by impregnation method for catalytic combustion of methane in air were investigated. The catalysts before and after reaction were characterized by BET, CO chemisorption, XRD and XP S techniques. Results showed that the presence of Ce significantly increased the activity and thermal stability of the Pd-Pt/Al2O3 catalyst towards methane combustion, which could be attributed to more highly-dispersed active PdO particles over the Pd-Pt/Ce/Al2O3 catalyst surface as well as the retarded sintering of PdO and the maintained oxidized state of surface Pd during the combustion process in the presence of Ce.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Aluminum Oxide / chemistry*
  • Catalysis
  • Cesium / chemistry*
  • Methane / chemistry
  • Palladium / chemistry*
  • Photoelectron Spectroscopy
  • Platinum / chemistry*
  • X-Ray Diffraction

Substances

  • Cesium
  • Platinum
  • Palladium
  • Aluminum Oxide
  • Methane