Illuminating the surface spin texture of the giant-Rashba quantum-well system Bi/Ag(111) by circularly polarized photoemission

Phys Rev Lett. 2012 May 4;108(18):186403. doi: 10.1103/PhysRevLett.108.186403. Epub 2012 May 2.

Abstract

We have mapped out the spin texture of a Bi/Ag surface alloy prepared on a thin Ag film by circularly polarized angle-resolved photoemission spectroscopy. A term proportional to ∇·A in the interaction Hamiltonian gives rise to strong surface photoexcitation, which interferes with a Rashba contribution to yield a pronounced circular dichroic effect in Bi/Ag. The dipole transition, often taken to be the only important photoexcitation mechanism, is actually negligible. A parameter-free calculation yields a dichroic pattern in excellent agreement with experiment.