Biodistribution of indocyanine green-loaded nanoparticles with surface modifications of PEG and folic acid

Int J Pharm. 2012 Oct 15;436(1-2):25-31. doi: 10.1016/j.ijpharm.2012.06.007. Epub 2012 Jun 9.

Abstract

Purpose: To establish the biodistribution profile of the PLGA nanoparticles with dual surface modifications of PEG and folic acid (FA) in mice xenografted with MDA-MB-231 human breast cancer cells with high expression of folate receptor (FR); and to illustrate that the modified nanoparticles can target the loaded indocyanine green (ICG) to the tumor with high FR expression.

Methods: ICG-loaded nanoparticles were prepared with PLGA (non-modified nanoparticles, NM-NP) or mPEG-PLGA and FA-PLGA (dual modified nanoparticles, DM-NP). Biodistribution of the ICG-loaded nanoparticles (1.25 mg/kg) after i.v. injection was investigated on athymic mice transplanted with MDA-MB-231 tumor.

Results: ICG concentration in plasma from the DM-NP group was significantly (p<0.05) higher than the NM-NP group from 90 min to the end of the study (12 h). After 4 h, the drug concentration in the tumor tissue from the DM-NP started to be significantly (p<0.05) higher than the NM-NP until 12 h. Compared to the NM-NP, the DM-NP increased the AUC(0-12 h) in plasma by 245% and the AUC(0-12 h) in tumor by 194%, while decreased the AUC(0-12 h) in liver by 13%.

Conclusion: The accumulation of DM-NP into the tumor was significantly higher than NM-NP due to the long circulation and FR-mediated uptake.

Publication types

  • Comparative Study

MeSH terms

  • Animals
  • Cell Line, Tumor
  • Coloring Agents / chemistry
  • Coloring Agents / pharmacokinetics*
  • Folic Acid / chemistry
  • Folic Acid / pharmacokinetics*
  • Humans
  • Indocyanine Green / chemistry
  • Indocyanine Green / pharmacokinetics*
  • Lactic Acid / chemistry
  • Lactic Acid / pharmacokinetics*
  • Mice
  • Mice, Nude
  • Nanoparticles / administration & dosage*
  • Nanoparticles / chemistry
  • Polyesters / chemistry
  • Polyesters / pharmacokinetics*
  • Polyethylene Glycols / chemistry
  • Polyethylene Glycols / pharmacokinetics*
  • Polyglycolic Acid / chemistry
  • Polyglycolic Acid / pharmacokinetics*
  • Polylactic Acid-Polyglycolic Acid Copolymer
  • Tissue Distribution

Substances

  • Coloring Agents
  • Polyesters
  • methoxypolyethyleneglycol-poly(lactic-co-glycolic acid)
  • Polylactic Acid-Polyglycolic Acid Copolymer
  • Polyglycolic Acid
  • Lactic Acid
  • Polyethylene Glycols
  • Folic Acid
  • Indocyanine Green