Interfacial catalysis: the mechanism of phospholipase A2

Science. 1990 Dec 14;250(4987):1541-6. doi: 10.1126/science.2274785.

Abstract

A chemical description of the action of phospholipase A2 (PLA2) can now be inferred with confidence from three high-resolution x-ray crystal structures. The first is the structure of the PLA2 from the venom of the Chinese cobra (Naja naja atra) in a complex with a phosphonate transition-state analogue. This enzyme is typical of a large, well-studied homologous family of PLA2S. The second is a similar complex with the evolutionarily distant bee-venom PLA2. The third structure is the uninhibited PLA2 from Chinese cobra venom. Despite the different molecular architectures of the cobra and bee-venom PLA2s, the transition-state analogue interacts in a nearly identical way with the catalytic machinery of both enzymes. The disposition of the fatty-acid side chains suggests a common access route of the substrate from its position in the lipid aggregate to its productive interaction with the active site. Comparison of the cobra-venom complex with the uninhibited enzyme indicates that optimal binding and catalysis at the lipid-water interface is due to facilitated substrate diffusion from the interfacial binding surface to the catalytic site rather than an allosteric change in the enzyme's structure. However, a second bound calcium ion changes its position upon the binding of the transition-state analogue, suggesting a mechanism for augmenting the critical electrophile.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Bee Venoms / analysis
  • Binding Sites
  • Calcium / metabolism
  • Catalysis
  • Chemical Phenomena
  • Chemistry, Physical
  • Elapid Venoms / analysis
  • Models, Molecular
  • Molecular Structure
  • Organophosphonates / metabolism
  • Phospholipases A / chemistry
  • Phospholipases A / metabolism*
  • Phospholipases A2
  • Phospholipids / metabolism
  • Protein Conformation
  • X-Ray Diffraction

Substances

  • Bee Venoms
  • Elapid Venoms
  • Organophosphonates
  • Phospholipids
  • Phospholipases A
  • Phospholipases A2
  • Calcium