Rapid screening of illicit additives in weight loss dietary supplements with desorption corona beam ionisation (DCBI) mass spectrometry

Food Addit Contam Part A Chem Anal Control Expo Risk Assess. 2012 Aug;29(8):1194-201. doi: 10.1080/19440049.2012.692395.

Abstract

Desorption corona beam ionisation (DCBI), the relatively novel ambient mass spectrometry (MS) technique, was utilised to screen for illicit additives in weight-loss food. The five usually abused chemicals - fenfluramine, N-di-desmethyl sibutramine, N-mono-desmethyl sibutramine, sibutramine and phenolphthalein - were detected with the proposed DCBI-MS method. Fast single-sample and high-throughput analysis was demonstrated. Semi-quantification was accomplished based on peak areas in the ion chromatograms. Four illicit additives were identified and semi-quantified in commercial samples. As there was no tedious sample pre-treatment compared with conventional HPLC methods, high-throughput analysis was achieved with DCBI. The results proved that DCBI-MS is a powerful tool for the rapid screening of illicit additives in weight-loss dietary supplements.

Publication types

  • Research Support, Non-U.S. Gov't
  • Validation Study

MeSH terms

  • Anti-Obesity Agents / chemistry*
  • Appetite Depressants / analysis
  • Appetite Depressants / chemistry
  • China
  • Chromatography, High Pressure Liquid
  • Cyclobutanes / analysis
  • Cyclobutanes / chemistry
  • Dietary Supplements / analysis*
  • Fenfluramine / analysis
  • Fenfluramine / chemistry
  • Food Contamination*
  • Food Inspection / methods*
  • Indicators and Reagents / analysis
  • Indicators and Reagents / chemistry
  • Legislation, Food
  • Mass Spectrometry
  • Phenolphthalein / analysis
  • Phenolphthalein / chemistry
  • Reproducibility of Results
  • Selective Serotonin Reuptake Inhibitors / analysis
  • Selective Serotonin Reuptake Inhibitors / chemistry

Substances

  • Anti-Obesity Agents
  • Appetite Depressants
  • Cyclobutanes
  • Indicators and Reagents
  • Serotonin Uptake Inhibitors
  • Fenfluramine
  • Phenolphthalein
  • sibutramine