Studies on the chemical modification of goat liver cystatin and the effect on its anti-papain inhibitory activity

J Fluoresc. 2012 Nov;22(6):1627-32. doi: 10.1007/s10895-012-1106-5. Epub 2012 Jul 26.

Abstract

Goat liver cystatin was subjected to various chemical modifications in order to ascertain the amino acid residues responsible for its structural and functional integrity. Modification of tryptophan by HNBB led to the complete inactivation of the protein. The inactivation was also accompanied by the complete loss of tryptophan fluorescence at 340 nm. The reaction of liver cystatin with HNBB yielded a characteristic decrease in absorbance at 280 nm. Acetylation of the amino groups of liver cystatin was carried out in the presence of acetic anhydride. The acetylated cystatin showed a decrease in fluorescence intensity at 335 nm which could be attributed to the modification of tyrosine residue due to side reaction.

MeSH terms

  • Absorption
  • Acetic Anhydrides / chemistry
  • Acetylation / drug effects
  • Animals
  • Cystatins / chemistry*
  • Cystatins / pharmacology*
  • Dose-Response Relationship, Drug
  • Goats*
  • Guanidine / pharmacology
  • Liver*
  • Oxidation-Reduction / drug effects
  • Papain / antagonists & inhibitors*
  • Protease Inhibitors / chemistry*
  • Protease Inhibitors / pharmacology*
  • Spectrometry, Fluorescence
  • Structure-Activity Relationship
  • Tryptophan / chemistry

Substances

  • Acetic Anhydrides
  • Cystatins
  • Protease Inhibitors
  • acetic anhydride
  • Tryptophan
  • Papain
  • Guanidine