Comparative study of the degradation of carbamazepine in water by advanced oxidation processes

Environ Technol. 2012 Jun;33(10-12):1101-9. doi: 10.1080/09593330.2011.610359.

Abstract

Degradation of carbamazepine (CBZ) using ultraviolet (UV), UV/H2O2, Fenton, UV/Fenton and photocatalytic oxidation with TiO2 (UV/TiO2) was studied in deionized water. The five different oxidation processes were compared for the removal kinetics of CBZ. The results showed that all the processes followed pseudo-first-order kinetics. The direct photolysis (UV alone) was found to be less effective than UV/H2O2 oxidation for the degradation of CBZ. An approximate 20% increase in the CBZ removal efficiency occurred with the UV/Fenton reaction as compared with the Fenton oxidation. In the UV/TiO2 system, the kinetics of CBZ degradation in the presence of different concentrations of TiO2 followed the pseudo-first order degradation, which was consistent with the Langmuir-Hinshelwood (L-H) model. On a time basis, the degradation efficiencies ofCBZ were in the following order: UV/Fenton (86.9% +/- 1.7%) > UV/TiO2 (70.4% +/- 4.2%) > Fenton (67.8% +/- 2.6%) > UV/H2O2 (40.65 +/- 5.1%) > UV (12.2% +/- 1.4%). However, the lowest cost was obtained with the Fenton process.

Publication types

  • Comparative Study
  • Evaluation Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Carbamazepine / chemistry*
  • Carbamazepine / radiation effects
  • Hydrogen Peroxide
  • Iron
  • Kinetics
  • Oxidation-Reduction
  • Photosensitizing Agents
  • Titanium
  • Ultraviolet Rays
  • Water Pollutants, Chemical / chemistry*
  • Water Pollutants, Chemical / radiation effects

Substances

  • Fenton's reagent
  • Photosensitizing Agents
  • Water Pollutants, Chemical
  • titanium dioxide
  • Carbamazepine
  • Hydrogen Peroxide
  • Titanium
  • Iron