Cobalt ion-mediated cysteine detection with a hyperbranched conjugated polyelectrolyte as a new sensing platform

Macromol Rapid Commun. 2012 Sep 26;33(18):1510-6. doi: 10.1002/marc.201200441. Epub 2012 Aug 9.

Abstract

A highly efficient colorimetric and fluorescence turn-off probe for the sensitive and selective detection of the biologically important amino acid, cysteine (Cys), is demonstrated using a newly synthesized water-soluble hyperbranched polymer (HP) containing sulfonic acid groups. The detection mechanism involves two steps: (i) the slight quenching of HP in the presence of Co(2+) in advance; and (ii) the gradual quenching of the HP-Co(2+) complex according to the concentration of Cys due to the absorption screening effect of the formation of the Cys-Co(2+) complex, which prevents HP from absorbing excitation energy.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biosensing Techniques / instrumentation*
  • Cobalt / chemistry*
  • Cysteine / chemistry*
  • Electrolytes / chemistry*
  • Ions / chemistry
  • Polymers / chemistry*

Substances

  • Electrolytes
  • Ions
  • Polymers
  • Cobalt
  • Cysteine