Purification and characterization of a recombinant β-D-xylosidase from Thermobifida fusca TM51

Protein J. 2012 Dec;31(8):641-50. doi: 10.1007/s10930-012-9440-7.

Abstract

The subject of our investigations was a recombinant β-D-xylosidase (TfBXyl43) from Thermobifida fusca TM51 which was expressed in E. coli BL21DE3 and was purified to apparent homogeneity. The SDS-PAGE investigations demonstrated that the molecular weight of the monomer unit is 62.5 kDa but the native-PAGE studies indicated that the mass of the enzyme is 240-250 kDa which proves the presence of a characteristic homo oligomer quaternary structure in solution phase. Optimal parameters of the enzyme activity were at pH 6.0 and 50 °C. The enzyme showed little stability under pH 4.5 and above 60 °C. The substrate specificity investigations indicated that the TfBXyl43 is an exo-glycosidase, hydrolyzing only xylobiose and -triose from the nonreducing end. Besides the enzyme shows very high specificity on the glycon part of the substrate, since it can only hydrolyze β-D-xylopyranoside derivatives. The importance of hydrophobic interactions in the binding of the substrates are supported that the enzyme can hydrolize about four times more efficiently the artificial p-nitrophenyl-β-D-xylopyranoside substrate compared to the natural one, xylobiose. Furthermore we could detect transxylosidase activity both in the case of xylobiose and p-nitrophenyl-β-D-xylopyranoside donors which is the first example among the inverting β-D-xylosidases from T. fusca.

MeSH terms

  • Actinomycetales / enzymology*
  • Actinomycetales / genetics
  • Bacterial Proteins / chemistry*
  • Bacterial Proteins / genetics
  • Bacterial Proteins / isolation & purification*
  • Bacterial Proteins / metabolism
  • Chromatography, Liquid
  • Enzyme Stability
  • Glycosides / metabolism
  • Hydrogen-Ion Concentration
  • Molecular Weight
  • Nuclear Magnetic Resonance, Biomolecular
  • Protein Conformation
  • Recombinant Proteins / chemistry
  • Recombinant Proteins / genetics
  • Recombinant Proteins / isolation & purification
  • Recombinant Proteins / metabolism
  • Substrate Specificity
  • Temperature
  • Xylosidases / chemistry*
  • Xylosidases / genetics
  • Xylosidases / isolation & purification*
  • Xylosidases / metabolism

Substances

  • Bacterial Proteins
  • Glycosides
  • Recombinant Proteins
  • 4-nitrophenyl beta-D-xyloside
  • Xylosidases
  • exo-1,4-beta-D-xylosidase