Sustained-release G-CSF microspheres using a novel solid-in-oil-in-oil-in-water emulsion method

Int J Nanomedicine. 2012:7:4559-69. doi: 10.2147/IJN.S33993. Epub 2012 Aug 17.

Abstract

Background: The main treatments for cancers are still chemotherapy and radiotherapy for intermediate-stage cancer and terminal cancer. However, the therapeutic methods often result in a decreased neutrophilic granulocyte count and other side effects. In this study, in order to improve the neutrophilic granulocyte levels in the blood after radiotherapy and chemotherapy, we developed a sustained-release granulocyte colony-stimulating factor (G-CSF) microsphere formulation using a novel solid-in-oil-in-oil-in-water (S/O/O/W) emulsification method.

Methods: G-CSF was loaded into dextran nanoparticles by freezing-induced phase separation, and then the G-CSF-loaded nanoparticles were encapsulated into sustained-release poly(lactic-co- glycolic acid) microspheres using S/O/O/W emulsification. The control microspheres were also prepared through W/O/W emulsification. The performance of the two microsphere formulations was investigated both in vitro and in vivo.

Results: The microspheres for the controlled release of G-CSF in a zero-order or near-zero-order pattern were provided for 2 weeks. The in vitro cumulative G-CSF release kept over 90% of its bioactivity, which was proved by a NFS-60 cell line growth assay. The microspheres of the control group fabricated by W/O/W emulsification maintained less then half of its bioactivity. The in vivo efficacy of microspheres made using the S/O/O/W method was higher than those using the W/O/W method.

Conclusion: These results suggested that the microspheres prepared by the S/O/O/W method had increased neutrophil activity compared to those prepared by W/O/W.

Keywords: G-CSF; bioactivity; microspheres; stability; sustained release.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cell Line, Tumor
  • Delayed-Action Preparations / chemistry
  • Delayed-Action Preparations / pharmacokinetics*
  • Delayed-Action Preparations / pharmacology
  • Dextrans / chemistry
  • Drug Stability
  • Emulsions / chemistry
  • Emulsions / pharmacokinetics*
  • Emulsions / pharmacology
  • Granulocyte Colony-Stimulating Factor / administration & dosage*
  • Granulocyte Colony-Stimulating Factor / chemistry
  • Granulocyte Colony-Stimulating Factor / pharmacokinetics*
  • Granulocyte Colony-Stimulating Factor / pharmacology
  • Kinetics
  • Male
  • Mice
  • Microspheres*
  • Nanoparticles / chemistry
  • Neutrophils / cytology
  • Neutrophils / drug effects
  • Oils / chemistry
  • Rats
  • Rats, Sprague-Dawley
  • Water / chemistry

Substances

  • Delayed-Action Preparations
  • Dextrans
  • Emulsions
  • Oils
  • Water
  • Granulocyte Colony-Stimulating Factor