Synthesis and characterization of a series of annelated benzotriazole based polymers with variable bandgap

J Org Chem. 2012 Nov 16;77(22):10035-41. doi: 10.1021/jo301281d. Epub 2012 Oct 31.

Abstract

Here we report the synthesis and characterization of a series of annelated benzotriazole based polymers with variable bandgap. Benzobistriazole monomers reported by us previously were desymmetrized using partial reduction ring opening followed by ring closure to produce a wide range of annelated benzotriazole based monomers. These monomers were co-polymerized with a fluorene moiety to give polymers with bandgaps ranging from 1.16 to 2.41 eV.