Inhibitory effects of tert-butylhydroquinone on osteoclast differentiation via up-regulation of heme oxygenase-1 and down-regulation of HMGB1 release and NFATc1 expression

J Appl Toxicol. 2014 Jan;34(1):49-56. doi: 10.1002/jat.2827. Epub 2012 Oct 30.

Abstract

Osteoclasts (OCLs) are multinucleated bone-resorbing cells that are differentiated by receptor activator of nuclear factor kappa-B ligand (RANKL) and macrophage colony-stimulating factor (M-CSF). Our recent studies have shown that heme-oxygenase-1 (HO-1), a stress-induced cytoprotective enzyme, plays an important role in OCL differentiation, although the pharmacological significance of this effect remains unknown. In this study, we investigated the effects of tert-butylhydroquinone (tBHQ), a pharmacological HO-1 inducer, on in vitro differentiation of bone marrow-derived macrophages (BMMs) or murine monocytic cell line RAW-D into OCLs. tBHQ inhibited the formation and the bone-resorbing activity of OCLs. Moreover, tBHQ treatment decreased the expression of nuclear factor of activated T cells cytoplasmic-1 (NFATc1), a master regulator of OCL differentiation, and of OCL markers transcriptionally regulated by NFATc1, such as Src and cathepsin K. In addition, tBHQ impaired phosphorylation of extracellular signal-regulated kinase, p38 mitogen-activated protein kinase (MAPK), Jun N-terminal kinase, Akt, and inhibitor of nuclear factor kappa B alpha (IκBα). Finally, we show that tBHQ inhibited the release of high mobility group box 1 (HMGB1), a recently identified activator of OCL differentiation. Thus, tBHQ inhibits OCL differentiation through the HO-1/HMGB1 pathways.

Keywords: heme oxygenase-1; high mobility group box 1; nuclear factor of activated T cells cytoplasmic-1; osteoclasts; tert-butylhydroquinone.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Cathepsin K / genetics
  • Cathepsin K / metabolism
  • Cell Differentiation / drug effects*
  • Down-Regulation / drug effects
  • HMGB1 Protein / genetics
  • HMGB1 Protein / metabolism*
  • Heme Oxygenase-1 / genetics
  • Heme Oxygenase-1 / metabolism*
  • Hydroquinones / pharmacology*
  • Macrophages / drug effects
  • Macrophages / metabolism
  • Male
  • Membrane Proteins / genetics
  • Membrane Proteins / metabolism*
  • Mice
  • Mice, Inbred BALB C
  • Monocytes / drug effects
  • Monocytes / metabolism
  • NFATC Transcription Factors / genetics
  • NFATC Transcription Factors / metabolism*
  • Osteoclasts / drug effects*
  • Osteoclasts / metabolism
  • Phosphorylation
  • Signal Transduction
  • Transcription Factors / genetics
  • Transcription Factors / metabolism
  • Up-Regulation / drug effects

Substances

  • HMGB1 Protein
  • HMGB1 protein, mouse
  • Hydroquinones
  • Membrane Proteins
  • NFATC Transcription Factors
  • Nfatc1 protein, mouse
  • Transcription Factors
  • 2-tert-butylhydroquinone
  • Heme Oxygenase-1
  • Hmox1 protein, mouse
  • Cathepsin K
  • Ctsk protein, mouse