Assessment of radiation damage in single-shot coherent diffraction of DNA molecules by an extreme-ultraviolet free-electron laser

Phys Rev E Stat Nonlin Soft Matter Phys. 2012 Oct;86(4 Pt 1):042901. doi: 10.1103/PhysRevE.86.042901. Epub 2012 Oct 25.

Abstract

We have investigated the progress of structural distortions in DNA molecules by single-shot coherent diffraction using extreme-ultraviolet radiation from a free-electron laser. A speckle pattern of DNA molecules was successfully acquired using photons in a single pulse with a 100 fs pulse width. The radiation damage was assessed by a cross correlation, revealing that the first exposure has significantly deformed most of the original structures. Molecules were not completely destroyed by the first single-shot exposure and underwent subsequent distortions through continued exposure, until eventually deforming into a radiation-hard structure.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Crystallography, X-Ray / methods
  • DNA / chemistry*
  • DNA / radiation effects*
  • Electrons
  • Lasers*
  • Microscopy / methods
  • Normal Distribution
  • Optics and Photonics
  • Photons
  • Radiation Protection / methods
  • Ultraviolet Rays

Substances

  • DNA