Anthraquinone-2-sulfonic acid (AQ2S) is a novel neurotherapeutic agent

Cell Death Dis. 2013 Jan 10;4(1):e451. doi: 10.1038/cddis.2012.187.

Abstract

Anthraquinone derivatives such as emodin have recently been shown to protect in models of beta amyloid β (Aβ) and tau aggregation-induced cell death. The mechanisms of action possibly involve preconditioning effects, anti-aggregation properties, and/or enhancing the phosphatidylinositol-3-kinase (PI3K)/AKT survival mechanism. We studied several natural (emodin, rhein, and aloin) and synthetic (AQ2S) anthraquinones, to screen for post-treatment therapeutic benefit in two models of neuronal death, namely hydrogen peroxide (H(2)O(2)) and staurosporine (STS)-induced injury. Treatment with emodin, rhein, or aloin failed to reduce H(2)O(2) injury. Moreover, consistent with emodin behaving like a mild toxin, it exacerbated oxidative injury at the highest concentration used (50 μM) in our post-treatment paradigm, and potently inhibited AKT. In contrast, AQ2S was neuroprotective. It reduced H(2)O(2) injury at 50 and 75 μM. In addition, AQ2S potently inhibited staurosporine (STS)-induced injury. The mechanisms of action involve caspase inhibition and AKT activation. However, blockade of AKT signaling with LY294002 failed to abolish AQ2S-mediated protection on the STS assay. This is the first study to report that AQ2S is a new neuroprotective compound and a novel caspase inhibitor.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Anthraquinones / chemistry
  • Anthraquinones / pharmacology*
  • Anthraquinones / therapeutic use
  • Apoptosis / drug effects
  • Caspases / chemistry
  • Caspases / metabolism
  • Cell Survival / drug effects
  • Cells, Cultured
  • Chromones / pharmacology
  • Emodin / analogs & derivatives
  • Emodin / chemistry
  • Emodin / pharmacology
  • Hydrogen Peroxide / toxicity
  • Lipid Peroxidation / drug effects
  • Morpholines / pharmacology
  • Neuroblastoma / drug therapy
  • Neuroblastoma / metabolism
  • Neuroblastoma / pathology
  • Neurons / cytology
  • Neurons / drug effects*
  • Neurons / metabolism
  • Neuroprotective Agents / chemistry
  • Neuroprotective Agents / pharmacology*
  • Neuroprotective Agents / therapeutic use
  • Oxidative Stress / drug effects
  • Proto-Oncogene Proteins c-akt / antagonists & inhibitors
  • Proto-Oncogene Proteins c-akt / metabolism
  • Rats
  • Rats, Sprague-Dawley
  • Staurosporine / toxicity

Substances

  • Anthraquinones
  • Chromones
  • Morpholines
  • Neuroprotective Agents
  • anthraquinone sulfonate
  • 2-(4-morpholinyl)-8-phenyl-4H-1-benzopyran-4-one
  • Hydrogen Peroxide
  • Proto-Oncogene Proteins c-akt
  • Caspases
  • Staurosporine
  • Emodin
  • alloin
  • rhein