Efficient production of 1,3-propanediol from glycerol upon constitutive expression of the 1,3-propanediol oxidoreductase gene in engineered Klebsiella pneumoniae with elimination of by-product formation

Bioprocess Biosyst Eng. 2013 Jun;36(6):757-63. doi: 10.1007/s00449-013-0901-y. Epub 2013 Jan 30.

Abstract

In the present study, we developed an efficient method of 1,3-propanediol (1,3-PD) production from glycerol by genetic engineering of Klebsiella pneumoniae AK mutant strains. The proposed approach eliminated by-product formation and IPTG induction resulted in maximal production of 1,3-PD. A series of recombinant strains was designed to constitutively express the dhaB and/or dhaT genes, using the bacteriophage T5 P(DE20) promoter and the rho-independent transcription termination signal of the Rahnella aquatilis levansucrase gene. Among these strains, AK/pConT expressing dhaT alone gave the highest yield of 1,3-PD. Fed-batch fermentation resulted in efficient production of 1,3-PD from either pure or crude glycerol, without by-product formation.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alcohol Dehydrogenase / biosynthesis*
  • Alcohol Dehydrogenase / genetics
  • Bacterial Proteins / biosynthesis*
  • Bacterial Proteins / genetics
  • Bacteriophages / genetics
  • Bacteriophages / metabolism
  • Cryoprotective Agents / metabolism
  • Cryoprotective Agents / pharmacology
  • Gene Expression*
  • Glycerol / metabolism*
  • Glycerol / pharmacology
  • Hexosyltransferases / biosynthesis
  • Hexosyltransferases / genetics
  • Klebsiella pneumoniae / genetics
  • Klebsiella pneumoniae / metabolism*
  • Metabolic Engineering*
  • Promoter Regions, Genetic
  • Propylene Glycols / metabolism*
  • Rahnella / enzymology
  • Rahnella / genetics
  • Viral Proteins / biosynthesis
  • Viral Proteins / genetics

Substances

  • Bacterial Proteins
  • Cryoprotective Agents
  • Propylene Glycols
  • Viral Proteins
  • 1,3-propanediol
  • Alcohol Dehydrogenase
  • 1,3-propanediol dehydrogenase
  • Hexosyltransferases
  • levansucrase
  • Glycerol