Channel- and angle-resolved above threshold ionization in the molecular frame

Phys Rev Lett. 2013 Jan 11;110(2):023004. doi: 10.1103/PhysRevLett.110.023004. Epub 2013 Jan 11.

Abstract

In strong-field ionization (SFI) of polyatomic molecules, the participation of multiple electronic ionization channels is emerging as a key aspect. In the molecular frame, each channel is expected to show a characteristic dependence of the SFI yield on the polarization direction of the ionizing field. We apply a new angle- and channel-resolved SFI technique to the polyatomic molecule 1,3-butadiene and compare these molecular-frame measurements with two leading theoretical models.