"Base effect" in the auto-tandem palladium-catalyzed synthesis of amino-substituted 1-methyl-1H-α-carbolines

Org Lett. 2013 Mar 1;15(5):1060-3. doi: 10.1021/ol400064r. Epub 2013 Feb 14.

Abstract

An auto-tandem Pd-catalyzed process consisting of an intramolecular direct arylation and an intermolecular Buchwald-Hartwig reaction for C-ring amino-substituted 1-methyl-1H-α-carboline synthesis has been developed. A mechanistic study of the direct arylation reaction revealed a rate effect of the inorganic base on the C-H activation step ("base effect"). The amines, reagents in the tandem protocol, appear to have a similar effect on the direct arylation.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amines / chemistry*
  • Carbolines / chemical synthesis*
  • Carbolines / chemistry
  • Catalysis
  • Indicators and Reagents
  • Molecular Structure
  • Palladium / chemistry*
  • Stereoisomerism

Substances

  • Amines
  • Carbolines
  • Indicators and Reagents
  • Palladium