A rational torsion sensing material was fabricated by wrapping aligned single-walled carbon nanotube (SWCNT) thin films onto the surface of a rod with a predetermined and fixed wrapping angle without destroying the internal network of the SWCNTs within the film. When applied as a torsion sensor, torsion could be measured up to 400 rad/meter, that is, more than 4 times higher than conventional optical fiber torsion sensors, by monitoring increases in resistance due to fracturing of the aligned SWCNT thin films.