The mechanism of inhibition by H2 of H2-evolution by hydrogenases

Chem Commun (Camb). 2013 Aug 7;49(61):6840-2. doi: 10.1039/c3cc43297a. Epub 2013 Jun 24.

Abstract

By analysing the results of experiments carried out with two FeFe hydrogenases and several "channel mutants" of a NiFe hydrogenase, we demonstrate that whether or not hydrogen evolution is significantly inhibited by H2 is not a consequence of active site chemistry, but rather relates to H2 transport within the enzyme.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Hydrogen / chemistry
  • Hydrogen / metabolism*
  • Hydrogenase / metabolism*
  • Iron-Sulfur Proteins / metabolism*
  • Models, Molecular

Substances

  • Iron-Sulfur Proteins
  • Hydrogen
  • iron hydrogenase
  • nickel-iron hydrogenase
  • Hydrogenase