A tubular one-dimensional polymer constructed from alternating clusters of europium(III)-water and copper(I) chloride bridged by 4-(pyridin-4-yl)benzoate

Acta Crystallogr C. 2013 Jul;69(Pt 7):712-5. doi: 10.1107/S0108270113014765. Epub 2013 Jun 8.

Abstract

A new 3d-4f heterometallic polymer, poly[[aqua-μ3-chlorido-[μ3-4-(pyridin-4-yl)benzoato]tris[μ2-4-(pyridin-4-yl)benzoato]dicopper(I)erbium(III)] dihydrate], {[Cu2Er(C12H8NO2)4Cl(H2O)]·2H2O}n, was synthesized by the hydrothermal reaction of Er2O3, CuCl2·2H2O and 4-(pyridin-4-yl)benzoic acid in the presence of HClO4. The asymmetric unit contains one Er(3+) cation, two Cu(+) cations, one Cl(-) anion, four deprotonated 4-(pyridin-4-yl)benzoate ligands, one coordinated aqua ligand and two solvent water molecules. This tubular one-dimensional polymer is constructed from alternating clusters of europium(III)-water and copper(I) chloride bridged by 4-(pyridin-4-yl)benzoate ligands. Extensive hydrogen-bonding interactions involving both the coordinated and the solvent water molecules provide further stabilization to the structure.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Benzoates / chemistry*
  • Copper / chemistry*
  • Crystallography, X-Ray
  • Europium / chemistry*
  • Hydrogen Bonding
  • Models, Molecular
  • Organometallic Compounds*
  • Polymers / chemistry*
  • Pyridines / chemistry*
  • Water / chemistry

Substances

  • Benzoates
  • Organometallic Compounds
  • Polymers
  • Pyridines
  • Water
  • Europium
  • Copper
  • cuprous chloride