Targeting mutant p53 by a SIRT1 activator YK-3-237 inhibits the proliferation of triple-negative breast cancer cells

Oncotarget. 2013 Jul;4(7):984-94. doi: 10.18632/oncotarget.1070.

Abstract

Many types of mutations in tumor suppressor p53 are oncogenic through gain-of-function. Therefore, targeting mutant p53 (mtp53) is a promising therapeutic approach to fight against many types of cancers. We report here a small molecule compound YK-3-237 that reduces acetylation of mtp53 and exhibits anti-proliferative effects toward triple-negative breast cancer (TNBC) cells carrying mtp53. YK-3-237 activates SIRT1 enzyme activities in vitro and deacetylation of both mtp53 in a SIRT1-dependent manner. Deacetylation of mtp53 resulted in depletion of mtp53 protein level and up-regulated the expression of WTp53-target genes, PUMA and NOXA. YK-3-237 also induces PARP-dependent apoptotic cell death and arrests the cell cycle at G2/M phase of mtp53 TNBC cells. Taken together, our data suggest that targeting acetylation of mtp53 is a potential target to treat human cancers.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acetylation / drug effects
  • Apoptosis / physiology
  • Boronic Acids / pharmacology*
  • Cell Line, Tumor
  • Cell Proliferation / drug effects
  • Chalcones / pharmacology*
  • Female
  • Gene Expression / drug effects
  • Humans
  • Molecular Targeted Therapy
  • RNA, Small Interfering / genetics
  • RNA, Small Interfering / metabolism
  • Sirtuin 1 / genetics
  • Sirtuin 1 / metabolism*
  • Transfection
  • Triple Negative Breast Neoplasms / drug therapy*
  • Triple Negative Breast Neoplasms / genetics
  • Triple Negative Breast Neoplasms / metabolism
  • Triple Negative Breast Neoplasms / pathology
  • Tumor Suppressor Protein p53 / genetics
  • Tumor Suppressor Protein p53 / metabolism*

Substances

  • Boronic Acids
  • Chalcones
  • RNA, Small Interfering
  • TP53 protein, human
  • Tumor Suppressor Protein p53
  • YK-3-237
  • SIRT1 protein, human
  • Sirtuin 1