Escherichia coli heptosyltransferase I: investigation of protein dynamics of a GT-B structural enzyme

Biochemistry. 2013 Aug 6;52(31):5158-60. doi: 10.1021/bi400807r. Epub 2013 Jul 23.

Abstract

Heptosyltransferase I (HepI), the enzyme responsible for the transfer of l-glycero-d-manno-heptose to a 3-deoxy-α-d-manno-oct-2-ulopyranosonic acid (Kdo) of the growing core region of lipopolysaccharide, is a member of the GT-B structural class of enzymes. Crystal structures have revealed open and closed conformations of apo and ligand-bound GT-B enzymes, implying that large-scale protein conformational dynamics play a role in their reaction mechanism. Here we report transient kinetic analysis of conformational changes in HepI reported by intrinsic tryptophan fluorescence and present the first real-time evidence of a GT-B enzyme undergoing a substrate binding-induced transition from an open to closed state prior to catalysis.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Crystallization
  • Escherichia coli / chemistry
  • Escherichia coli / enzymology*
  • Escherichia coli / genetics
  • Escherichia coli Proteins / chemistry*
  • Escherichia coli Proteins / genetics
  • Escherichia coli Proteins / metabolism
  • Glycosyltransferases / chemistry*
  • Glycosyltransferases / genetics
  • Glycosyltransferases / metabolism
  • Kinetics
  • Protein Binding
  • Protein Conformation
  • Substrate Specificity

Substances

  • Escherichia coli Proteins
  • Glycosyltransferases
  • heptosyltransferase