Near-edge x-ray absorption fine structures revealed in core ionization photoelectron spectroscopy

Phys Rev Lett. 2013 Sep 20;111(12):123001. doi: 10.1103/PhysRevLett.111.123001. Epub 2013 Sep 20.

Abstract

Simultaneous core ionization and core excitation have been observed in the C(2)H(2n) (n=1, 2, 3) molecular series using synchrotron radiation and a magnetic bottle time-of-flight electron spectrometer. Rich satellite patterns corresponding to (K(-2)V) core excited states of the K(-1) molecular ions have been identified by detecting in coincidence the photoelectron with the two Auger electrons resulting from the double core hole relaxation. A theoretical model is proposed providing absolute photoionization cross sections and revealing clear signatures of direct (monopolar) and conjugate (dipolar near-edge x-ray absorption fine structure) shakeup lines of comparable magnitude.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Hydrocarbons / chemistry*
  • Photoelectron Spectroscopy / methods*
  • X-Ray Absorption Spectroscopy / methods*

Substances

  • Hydrocarbons