Effect of coumarin derivative-mediated inhibition of P-glycoprotein on oral bioavailability and therapeutic efficacy of paclitaxel

Eur J Pharmacol. 2014 Jan 15:723:381-8. doi: 10.1016/j.ejphar.2013.11.002. Epub 2013 Nov 16.

Abstract

Since P-glycoprotein (P-gp) acts as a barrier to intestinal absorption of various drugs, P-gp inhibitors have been studied as oral absorption enhancers of P-gp substrate drugs. Here, we investigated the in vitro and in vivo effects of a novel coumarin derivative (LL-348) for its P-gp inhibitory activity. With LL-348, accumulation of daunomycin (DNM) increased 270% and efflux of DNM decreased 63% compared to that of DNM alone. Paclitaxel (PTX, 25mg/kg) after oral administration with LL-348 (5mg/kg), the optimal dose of LL-348 as an oral absorption enhancer of PTX, improved the relative bioavailability (RB) of PTX to 961%. In a xenograft animal model, PTX (40mg/kg) treated with LL-348 (10mg/kg) significantly increased the efficacy of PTX. The results collectively demonstrate that LL-348 can provide a therapeutic benefit in the oral absorption of P-gp substrate anticancer drugs.

Keywords: Bioavailability; Coumarin derivative; Daunomycin; P-glycoprotein; Paclitaxel; Xenograft.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • ATP Binding Cassette Transporter, Subfamily B, Member 1 / antagonists & inhibitors
  • Administration, Oral
  • Animals
  • Antibiotics, Antineoplastic / pharmacology
  • Antineoplastic Agents, Phytogenic / blood
  • Antineoplastic Agents, Phytogenic / pharmacokinetics*
  • Antineoplastic Agents, Phytogenic / therapeutic use*
  • Biological Availability
  • Cell Line, Tumor
  • Cell Survival / drug effects
  • Coumarins / pharmacology*
  • Daunorubicin / pharmacology
  • Humans
  • Male
  • Mice
  • Mice, Nude
  • Neoplasms / drug therapy
  • Neoplasms / pathology
  • Paclitaxel / blood
  • Paclitaxel / pharmacokinetics*
  • Paclitaxel / therapeutic use*
  • Rats
  • Rats, Sprague-Dawley
  • Treatment Outcome
  • Tumor Burden / drug effects
  • Xenograft Model Antitumor Assays

Substances

  • ATP Binding Cassette Transporter, Subfamily B, Member 1
  • Antibiotics, Antineoplastic
  • Antineoplastic Agents, Phytogenic
  • Coumarins
  • Paclitaxel
  • Daunorubicin