Structural and binding properties of the PASTA domain of PonA2, a key penicillin binding protein from Mycobacterium tuberculosis

Biopolymers. 2014 Jul;101(7):712-9. doi: 10.1002/bip.22447.

Abstract

PonA2 is one of the two class A penicillin binding proteins of Mycobacterium tuberculosis, the etiologic agent of tuberculosis. It plays a complex role in mycobacterial physiology and is spotted as a promising target for inhibitors. PonA2 is involved in adaptation of M. tuberculosis to dormancy, an ability which has been attributed to the presence in its sequence of a C-terminal PASTA domain. Since PASTA modules are typically considered as β-lactam antibiotic binding domains, we determined the solution structure of the PASTA domain from PonA2 and analyzed its binding properties versus a plethora of potential binders, including the β-lactam antibiotics, two typical muropeptide mimics, and polymeric peptidoglycan. We show that, despite a high structural similarity with other PASTA domains, the PASTA domain of PonA2 displays different binding properties, as it is not able to bind muropeptides, or β-lactams, or polymeric peptidoglycan. These results indicate that the role of PASTA domains cannot be generalized, as their specific binding properties strongly depend on surface residues, which are widely variable.

Keywords: binding; structure; tuberculosis.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Bacterial Proteins / chemistry*
  • Bacterial Proteins / metabolism
  • Calorimetry / methods
  • Circular Dichroism
  • Magnetic Resonance Spectroscopy / methods
  • Models, Molecular
  • Mycobacterium tuberculosis / metabolism*
  • Penicillin-Binding Proteins / chemistry*
  • Penicillin-Binding Proteins / metabolism
  • Peptidoglycan / chemistry
  • Peptidoglycan / metabolism
  • Protein Binding
  • Protein Structure, Tertiary*
  • Protein Unfolding
  • Temperature
  • beta-Lactams / chemistry
  • beta-Lactams / metabolism

Substances

  • Bacterial Proteins
  • Penicillin-Binding Proteins
  • Peptidoglycan
  • beta-Lactams