Digitally enhanced thin layer chromatography: further development and some applications in isotopic chemistry

J Labelled Comp Radiopharm. 2013 Sep;56(11):544-52. doi: 10.1002/jlcr.3052. Epub 2013 Jul 23.

Abstract

Improvements to thin layer chromatography (TLC) analysis can be made easily and cheaply by the application of digital colour photography and image analysis. The combined technique, digitally enhanced TLC (DE-TLC), is applicable to the accurate quantification of analytes in mixtures, to reaction monitoring and to other typical uses of TLC. Examples are given of the application of digitally enhanced TLC to: the deuteromethylations of theophylline to [methyl-(2)H3]caffeine and of umbelliferone to [(2)H3]7-methoxycoumarin; the selection of tertiary amine bases in deuterodechlorination reactions; stoichiometry optimisation in the borodeuteride reduction of quinizarin (1,4-dihydroxyanthraquinone) and to the assessment of xanthophyll yields in Lepidium sativum seedlings grown in deuterated media.

Keywords: DE-TLC; Lepidium sativum carotenoids; [2H3]7-methoxycoumarin; [9,10−2H2]1,4-anthraquinone; deuteromethylation; digitally enhanced TLC; methyl−2H3]caffeine; quinizarin; umbelliferone.

MeSH terms

  • Anthraquinones / analysis
  • Caffeine / analogs & derivatives
  • Caffeine / analysis
  • Carotenoids / analysis
  • Chromatography, Thin Layer / methods*
  • Image Processing, Computer-Assisted / methods*
  • Isotope Labeling / methods
  • Lepidium sativum / chemistry
  • Sensitivity and Specificity
  • Theophylline / analysis
  • Tritium / analysis*

Substances

  • 2-methylcaffeine
  • Anthraquinones
  • Tritium
  • Carotenoids
  • Caffeine
  • 1,4-dihydroxyanthraquinone
  • Theophylline