Detection and quantification of dermorphin and selected analogs in equine urine

Bioanalysis. 2013 Dec;5(24):2995-3007. doi: 10.4155/bio.13.281.

Abstract

Background: Dermorphin, a hepta-peptide with potent analgesic properties, is classified as a doping agent in equine racing. Since its discovery, a number of biologically active structural analogs have been synthesized and made commercially available so there is a need for reliable methods of detection.

Methodology/results: A sensitive detection method was developed for dermorphin and six analogs in equine urine. Peptide enrichment was achieved using weak cation exchange with subsequent separation and detection by nano-UHPLC-MS/MS. Method validation parameters included: specificity, linearity (5-10000 pg/ml), recovery (58-93%), intra and inter-assay repeatability, LOD (5-50 pg/ml) and matrix effects.

Conclusion: The presented method will facilitate the control of the abuse of dermorphin and selected analogs in equine sports.

Publication types

  • Research Support, Non-U.S. Gov't
  • Validation Study

MeSH terms

  • Analgesics, Opioid / analysis
  • Analgesics, Opioid / urine*
  • Animals
  • Chromatography, High Pressure Liquid / methods
  • Chromatography, High Pressure Liquid / veterinary*
  • Horses / urine*
  • Limit of Detection
  • Opioid Peptides / analysis
  • Opioid Peptides / urine*
  • Substance Abuse Detection / methods
  • Substance Abuse Detection / veterinary*
  • Tandem Mass Spectrometry / methods
  • Tandem Mass Spectrometry / veterinary*

Substances

  • Analgesics, Opioid
  • Opioid Peptides
  • dermorphin