Structure-dependent binding of arylimidamides to the DNA minor groove

Chembiochem. 2014 Jan 3;15(1):68-79. doi: 10.1002/cbic.201300622. Epub 2013 Dec 9.

Abstract

Heterocyclic diamidines are strong DNA minor-groove binders and have excellent antiparasitic activity. To extend the biological activity of these compounds, a series of arylimidamides (AIAs) analogues, which have better uptake properties in Leishmania and Trypanosoma cruizi than diamidines, was prepared. The binding of the AIAs to DNA was investigated by Tm , fluorescence displacement titration, circular dichroism, DNase I footprinting, biosensor surface plasmon resonance, X-ray crystallography and molecular modeling. These compounds form 1:1 complexes with AT sequences in the DNA minor groove, and the binding strength varies with substituent size, charge and polarity. These substituent-dependent structure and properties provide a SAR that can be used to estimate K values for binding to DNA in this series. The structural results and molecular modeling studies provide an explanation for the differences in binding affinities for AIAs.

Keywords: DNA; X-ray crystallography; arylimidamides; minor-groove binders; molecular modeling.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amides / chemistry
  • Amides / metabolism*
  • Base Sequence
  • Binding Sites
  • Circular Dichroism
  • Crystallography, X-Ray
  • DNA / chemistry
  • DNA / metabolism*
  • Deoxyribonuclease I / metabolism
  • Leishmania / metabolism
  • Molecular Docking Simulation
  • Nucleic Acid Conformation
  • Substrate Specificity
  • Surface Plasmon Resonance
  • Transition Temperature
  • Trypanosoma cruzi / metabolism

Substances

  • Amides
  • DNA
  • Deoxyribonuclease I