In-filter PCDF and PCDD formation at low temperature during MSWI combustion

Chemosphere. 2014 May:102:12-7. doi: 10.1016/j.chemosphere.2013.11.068. Epub 2013 Dec 18.

Abstract

This case study investigated PCDF and PCDD emissions from a 65 MW waste-to-energy plant to identify why an air pollution control system remodeling to accommodate increased production resulted in increased TEQ concentrations. Pre- and post-filter gases were collected simultaneously in four sample sets with varying filter temperatures and with/without activated carbon injection. Samples were analyzed to determine total PCDF and PCDD concentrations, as well as homologue profiles, and concentrations of individual congeners (some remained co-eluted). The total post filter PCDD concentrations where found to increase while the concentrations of PCDF and 2,3,7,8-substituted congeners declined. An investigation of the individual congener concentrations revealed that the increase of PCDD concentrations were due to a few congeners, suggesting a single formation route. The study also concludes that vital information about the formation could be obtained by not restricting the analysis to just the 2,3,7,8-substituted congeners.

Keywords: Case study; Fabric filters; Full scale; MSWI; PCDD; PCDF.

MeSH terms

  • Air Pollution / prevention & control*
  • Benzofurans / analysis*
  • Cold Temperature
  • Conservation of Natural Resources
  • Dibenzofurans, Polychlorinated
  • Filtration
  • Gases
  • Incineration*
  • Polychlorinated Dibenzodioxins / analogs & derivatives*
  • Polychlorinated Dibenzodioxins / analysis
  • Temperature

Substances

  • Benzofurans
  • Dibenzofurans, Polychlorinated
  • Gases
  • Polychlorinated Dibenzodioxins