Oxoglaucine-lanthanide complexes: synthesis, crystal structure and cytotoxicity

Anticancer Res. 2014 Jan;34(1):531-6.

Abstract

Aim: To evaluate the in vitro cytotoxicity of oxoglaucine (OG) complexes: [Sm(OG)2(NO3)3]•H2O (1), [Eu(OG)2(NO3)3]•1.5CH3OH (2) and [Er(OG)2(NO3)3]•H2O (3) through comparison to oxoglaucine and lanthanide salts.

Materials and methods: The reactions of OG with corresponding lanthanide salts gave rise to complexes 1-3. The crystal structures of complexes 1-3 were determined by single-crystal X-ray diffraction analysis. The in vitro cytotoxicity of oxoglaucine and complexes 1-3 against five human cancer cell lines were evaluated by the 3-(4,5-dimethyl-2-thiazolyl)-2,5-diphenyl tetrazolium Bromide (MTT) method.

Results: Complexes 1-3 have similar mononuclear structures. The 50% inhibitory concentration (IC50) of complex 1 against SGC7901 cells was 32.1 μM; that of complex 2 against MCF-7 cells was 3.2 μM; those of complex 3 on HeLa and MCF-7 cells were 8.3 and 1.4 μM, respectively.

Conclusion: The three OG-lanthanide complexes exhibited significantly enhanced cytotoxicity vs. OG and corresponding lanthanide salts.

Keywords: Lanthanide complex; crystal structure; cytotoxicity; oxoglaucine.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Apomorphine / analogs & derivatives*
  • Apomorphine / chemistry
  • Apomorphine / pharmacology
  • Apoptosis / drug effects*
  • Crystallography, X-Ray
  • Humans
  • Inhibitory Concentration 50
  • Lanthanoid Series Elements / chemistry*
  • Lanthanoid Series Elements / pharmacology*
  • Models, Molecular
  • Neoplasms / drug therapy*
  • Neoplasms / pathology
  • Tumor Cells, Cultured

Substances

  • Lanthanoid Series Elements
  • oxoglaucine
  • Apomorphine