Total synthesis of sulfolipid-1

Chem Commun (Camb). 2014 Mar 4;50(18):2286-8. doi: 10.1039/c3cc48087a. Epub 2014 Jan 17.

Abstract

Sulfolipid-1, a tetra-acylated sulfotrehalose from Mycobacterium tuberculosis, was isolated over 40 years ago. Being a main component of the mycomembrane of M. tuberculosis, its biosynthesis and function have been studied in depth, but the chemical synthesis of sulfolipid-1 has not been reported. The synthesis presented here is based on iterative catalytic asymmetric conjugate additions of methylmagnesium bromide for the preparation of the phthioceranic and hydroxyphthioceranic acid side chains, a double regioselective reductive ring-opening and a fivefold deprotection in the final step.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Glycolipids / chemical synthesis*
  • Glycolipids / chemistry
  • Molecular Conformation
  • Mycobacterium tuberculosis / chemistry
  • Virulence Factors / chemical synthesis*
  • Virulence Factors / chemistry

Substances

  • Glycolipids
  • Virulence Factors
  • sulfolipid I