Catalytic nanoreactors in continuous flow: hydrogenation inside single-walled carbon nanotubes using supercritical CO2

Chem Commun (Camb). 2014 May 25;50(40):5200-2. doi: 10.1039/c3cc49247h. Epub 2014 Feb 5.

Abstract

One nanometre wide carbon nanoreactors are utilised as the reaction vessel for catalytic chemical reactions on a preparative scale. Sub-nanometre ruthenium catalytic particles which are encapsulated solely within single-walled carbon nanotubes offering a unique reaction environment are shown to be active when embedded in a supercritical CO2 continuous flow reactor. A range of hydrogenation reactions were tested and the catalyst displayed excellent stability over extended reaction times.