Resolving ultrafast heating of dense cryogenic hydrogen

Phys Rev Lett. 2014 Mar 14;112(10):105002. doi: 10.1103/PhysRevLett.112.105002. Epub 2014 Mar 12.

Abstract

We report on the dynamics of ultrafast heating in cryogenic hydrogen initiated by a ≲300 fs, 92 eV free electron laser x-ray burst. The rise of the x-ray scattering amplitude from a second x-ray pulse probes the transition from dense cryogenic molecular hydrogen to a nearly uncorrelated plasmalike structure, indicating an electron-ion equilibration time of ∼0.9 ps. The rise time agrees with radiation hydrodynamics simulations based on a conductivity model for partially ionized plasma that is validated by two-temperature density-functional theory.