Palladium-catalyzed cross-coupling reactions of arylsiloxanes with aryl halides: application to solid-supported organic synthesis

ACS Comb Sci. 2014 May 12;16(5):211-4. doi: 10.1021/co5000322. Epub 2014 Apr 7.

Abstract

The solid-phase version of the Pd-catalyzed Hiyama reaction between a variety of aryltriethoxysilanes and immobilized aryl halides was developed. Smooth cross-coupling was achieved to afford the corresponding biaryl products in moderate to excellent yields. The described protocol would be particularly useful for the construction of 4'-substituted 1,1'-biphenyl derivatives.

Keywords: Hiyama coupling; cross-coupling reactions; solid-phase organic synthesis.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biphenyl Compounds / chemical synthesis*
  • Biphenyl Compounds / chemistry
  • Catalysis
  • Palladium / chemistry*
  • Silanes / chemical synthesis
  • Silanes / chemistry*
  • Solid-Phase Synthesis Techniques / methods*

Substances

  • Biphenyl Compounds
  • Silanes
  • diphenyl
  • Palladium