Effects of Asn-33 glycosylation on the thermostability of Thermomyces lanuginosus lipase

J Appl Microbiol. 2014 Jul;117(1):151-9. doi: 10.1111/jam.12519. Epub 2014 May 2.

Abstract

Aims: The study was to examine whether glycosylation could improve the thermostability of recombinant Thermomyces lanuginosus lipase (Tll) expressed in Pichia pastoris.

Methods and results: The Tll gene was synthesized and transformed into Pichia pastoris GS115.The recombinant Tll protein was expressed and purified, and its glycosylation site was identified by LCMS/MS as Asn-33. Two nonglycosylated mutants were constructed and the variant proteins were also expressed and purified. Effects of temperature on activities of the wild-type Tll and variants were analysed. The glycosylated Tll exhibited better thermostability than nonglycosylated variants.

Conclusions: Our experiments have demonstrated the improvement of Tll thermostability by Asn-33 glycosylation.

Significance and impact of the study: This work has deepened our understanding in the mechanism of Tll thermostability and will guide us to directional improvement of lipases and even other industrial enzymes.

Keywords: Thermomyces lanuginosus lipase; glycosylation; mutation; thermostability.

MeSH terms

  • Asparagine / metabolism*
  • Fungal Proteins / genetics
  • Fungal Proteins / metabolism*
  • Gene Expression
  • Glycosylation
  • Lipase / genetics
  • Lipase / metabolism*
  • Molecular Sequence Data
  • Pichia / enzymology
  • Pichia / genetics*
  • Protein Stability
  • Recombinant Proteins / genetics
  • Recombinant Proteins / metabolism
  • Saccharomycetales / chemistry*
  • Saccharomycetales / enzymology
  • Temperature

Substances

  • Fungal Proteins
  • Recombinant Proteins
  • Asparagine
  • Lipase

Associated data

  • GENBANK/AF054513