Metal-free oxidative synthesis of quinazolinones via dual amination of sp3 C-H bonds

Chem Commun (Camb). 2014 Jun 21;50(49):6471-4. doi: 10.1039/c4cc02648a. Epub 2014 May 9.

Abstract

A novel metal-free synthesis of quinazolinones via dual amination of sp(3) C-H bonds was developed. The sp(3) carbon in methylarenes or adjacent to a heteroatom in DMSO, DMF or DMA was used as the one carbon synthon.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amination
  • Benzenesulfonates / chemistry
  • Carbon / chemistry*
  • Hydrogen / chemistry*
  • Metals / chemistry
  • Oxidation-Reduction
  • Quantum Theory
  • Quinazolinones / chemical synthesis
  • Quinazolinones / chemistry*
  • Solvents / chemistry

Substances

  • Benzenesulfonates
  • Metals
  • Quinazolinones
  • Solvents
  • Carbon
  • Hydrogen
  • 4-toluenesulfonic acid