Spectroscopy and energy transfer in lead borate glasses doubly doped with Dy(3)(+)-Tb(3+) and Tb(3)(+)-Eu(3+) ions

Spectrochim Acta A Mol Biomol Spectrosc. 2014 Aug 14:129:649-53. doi: 10.1016/j.saa.2014.04.142. Epub 2014 May 2.

Abstract

Lead borate glasses doubly doped with Dy(3)(+)-Tb(3+) and Tb(3+)-Eu(3+) were investigated using optical spectroscopy. Luminescence spectra of rare earths were detected under various excitation wavelengths. The main green emission band due to (5)D4→(7)F5 transition of Tb(3+) is observed under excitation of Dy(3+), whereas the main red emission band related to (5)D0→(7)F2 transition of Eu(3+) is successfully observed under direct excitation of Tb(3+). In both cases, the energy transfer processes from Dy(3+) to Tb(3+) and from Tb(3+) to Eu(3+) in lead borate glasses occur through a nonradiative processes with efficiencies up to 16% and 18%, respectively. The presence of energy transfer process was also confirmed by excitation spectra measurements.

Keywords: Energy transfer processes; Lead borate glasses; Luminescence; Rare earth ions.

MeSH terms

  • Borates / chemistry*
  • Cations / chemistry
  • Dysprosium / chemistry*
  • Energy Transfer
  • Europium / chemistry*
  • Glass / chemistry*
  • Lead / chemistry*
  • Luminescence
  • Terbium / chemistry*

Substances

  • Borates
  • Cations
  • Terbium
  • Dysprosium
  • Lead
  • Europium