Isolation, structural elucidation and anti-inflammatory activity of astragalin, (-)hinokinin, aristolactam I and aristolochic acids (I & II) from Aristolochia indica

Nat Prod Res. 2014;28(17):1413-7. doi: 10.1080/14786419.2014.905563. Epub 2014 May 23.

Abstract

Astragalin was isolated for the first time along with (-)hinokinin, aristolactam I and aristolochic acids (I & II) from the extracts of Aristolochia indica L. using a new, efficient preparative HPLC method. A reversed-phase HPLC method of analysis was developed to analyse the isolated compounds. The crude extracts and the isolated compounds were tested for their anti-inflammatory potential. We report here for the first time the anti-inflammatory effects of (-)hinokinin and aristolactam I against IL-6 (IC50 = 20.5 ± 0.5 and 52 ± 8 μM) and TNFα (IC50 = 77.5 ± 27.5 and 116.8 ± 83.25 μM), respectively. (-)Hinokinin exerted its anti-inflammatory effects via NFκB-dependent mechanism whereas aristolactam I may be effective via a mechanism independent of NFκB.

Keywords: ( − )hinokinin; Aristolochia indica; IL-6; NFκB; TNFα; aristolactam I; astragalin.

MeSH terms

  • 4-Butyrolactone / analogs & derivatives*
  • 4-Butyrolactone / chemistry
  • 4-Butyrolactone / isolation & purification
  • 4-Butyrolactone / pharmacology
  • Anti-Inflammatory Agents
  • Aristolochia / chemistry*
  • Aristolochic Acids / chemistry
  • Aristolochic Acids / isolation & purification*
  • Aristolochic Acids / pharmacology*
  • Benzodioxoles
  • Chromatography, High Pressure Liquid
  • Dioxoles / chemistry
  • Dioxoles / isolation & purification*
  • Dioxoles / pharmacology*
  • Interleukin-6 / antagonists & inhibitors
  • Kaempferols / chemistry
  • Kaempferols / isolation & purification*
  • Kaempferols / pharmacology*
  • Lignans / chemistry
  • Lignans / isolation & purification*
  • Lignans / pharmacology*

Substances

  • Anti-Inflammatory Agents
  • Aristolochic Acids
  • Benzodioxoles
  • Dioxoles
  • Interleukin-6
  • Kaempferols
  • Lignans
  • aristolactam I
  • hinokinin
  • astragalin
  • 4-Butyrolactone