Mesoporous amorphous FePO4 nanospheres as high-performance cathode material for sodium-ion batteries

Nano Lett. 2014 Jun 11;14(6):3539-43. doi: 10.1021/nl501152f. Epub 2014 May 28.

Abstract

FePO4 nanospheres are synthesized successfully through a simple chemically induced precipitation method. The nanospheres present a mesoporous amorphous structure. Electrochemical experiments show that the FePO4/C electrode demonstrates a high initial discharging capacity of 151 mAh g(-1) at 20 mA g(-1), stable cyclablilty (94% capacity retention ratio over 160 cycles), as well as high rate capability (44 mAh g(-1) at 1000 mA g(-1)) for Na-ion storage. The superior electrochemical performance of the FePO4/C nanocomposite is due to its particular mesoporous amorphous structure and close contact with the carbon framework, which significantly improve the ionic and electronic transport and intercalation kinetics of Na ions.

Publication types

  • Research Support, Non-U.S. Gov't