Preparation and characterization of a novel aspirin derivative with anti-thrombotic and gastric mucosal protection properties

PLoS One. 2014 Jun 3;9(6):e98513. doi: 10.1371/journal.pone.0098513. eCollection 2014.

Abstract

The use of acetylsalicylic acid (ASP) is limited by its adverse effects, especially the effect on the gastric mucosa. To address this problem, we synthesized a derivative form of ASP, prepared by modification of ASP with nano-hydroxyapatite (a kind of inorganic particle containing Ca(2+)). The derivative was named Ca-ASP. Structural study showed that Ca-ASP was a kind of carboxylate containing intramolecular hydrogen bonds. Rats given a high dose of Ca-ASP (5 mmol per kg body weight) showed similar anti-thrombotic activity as those given the same dose of ASP, but had much lower gastric mucosal damage than ASP (UI: 2 versus UI: 12.5). These rats also showed reduced expression of COX-2, but their COX-1 expression was similar to that of control rats, but significantly higher than that of ASP-administered rats. Furthermore, the level of prostaglandin E2 (PGE2) was up-regulated in Ca-ASP-administered rats compared to ASP-administered rats. Taken together, the results showed that Ca-ASP possessed similar antithrombotic activity as ASP but without the side effect associated with ASP, and the underlying mechanism may center on inhibiting COX-2 without inhibiting COX-1, and thus favouring the production of PGE2, the prostaglandin that plays a vital role in the suppression of platelet aggregation and thrombosis, as well as in the repair of gastric damage.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Aspirin / analogs & derivatives
  • Aspirin / pharmacology*
  • Cyclooxygenase 1 / genetics
  • Cyclooxygenase 1 / metabolism
  • Cyclooxygenase 2 / genetics
  • Cyclooxygenase 2 / metabolism
  • Dinoprostone / genetics
  • Dinoprostone / metabolism
  • Female
  • Gastric Mucosa / drug effects
  • Gastric Mucosa / metabolism*
  • Male
  • Rats
  • Rats, Wistar
  • Spectroscopy, Fourier Transform Infrared

Substances

  • Cyclooxygenase 1
  • Cyclooxygenase 2
  • Dinoprostone
  • Aspirin

Grants and funding

This work was financially supported by the Heilongjiang Young Scientists Fund of Natural Science Foundation (QC2011C099), Post-Doctoral Scientific Research Startup Fund (LBH-Q13131), and Postgraduate Innovation Scientific Research Fund YJSCX2012-212HLJ. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript.