High-temperature calcined fullerene nanowhiskers as well as long needle-like multi-wall carbon nanotubes have abilities to induce NLRP3-mediated IL-1β secretion

Biochem Biophys Res Commun. 2014 Sep 26;452(3):593-9. doi: 10.1016/j.bbrc.2014.08.118. Epub 2014 Aug 30.

Abstract

Because multi-wall carbon nanotubes (MWCNTs) have asbestos-like shape and size, concerns about their pathogenicity have been raised. Contaminated metals of MWCNTs may also be responsible for their toxicity. In this study, we employed high-temperature calcined fullerene nanowhiskers (HTCFNWs), which are needle-like nanofibers composed of amorphous carbon having similar sizes to MWCNTs but neither metal impurities nor tubular structures, and investigated their ability to induce production a major proinflammatory cytokine IL-1β via the Nod-like receptor pyrin domain containing 3 (NLRP3)-containing flammasome-mediated mechanism. When exposed to THP-1 macrophages, long-HTCFNW exhibited robust IL-1β production as long and needle-like MWCNTs did, but short-HTCFNW caused very small effect. IL-1β release induced by long-HTCFNW as well as by long, needle-like MWCNTs was abolished by a caspase-1 inhibitor or siRNA-knockdown of NLRP3, indicating that NLRP3-inflammasome-mediated IL-1β production by these carbon nanofibers. Our findings indicate that the needle-like shape and length, but neither metal impurities nor tubular structures of MWCNTs were critical to robust NLRP3 activation.

Keywords: Carbon nanotubes; Fullerene nanowhiskers; IL-1β; NLRP3.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Chloromethyl Ketones / pharmacology
  • Carrier Proteins / antagonists & inhibitors
  • Carrier Proteins / genetics*
  • Carrier Proteins / metabolism
  • Caspase 1 / genetics
  • Caspase 1 / metabolism
  • Caspase Inhibitors / pharmacology
  • Cell Line
  • Fullerenes / chemistry
  • Fullerenes / pharmacology*
  • Gene Expression
  • Hot Temperature
  • Humans
  • Inflammasomes / drug effects
  • Inflammasomes / metabolism
  • Interleukin-1beta / biosynthesis
  • Interleukin-1beta / metabolism*
  • Macrophages / cytology
  • Macrophages / drug effects*
  • Macrophages / metabolism
  • NLR Family, Pyrin Domain-Containing 3 Protein
  • Nanofibers / chemistry
  • Nanofibers / toxicity*
  • Nanotubes, Carbon / chemistry
  • Nanotubes, Carbon / toxicity*
  • RNA, Small Interfering / genetics
  • RNA, Small Interfering / metabolism

Substances

  • Amino Acid Chloromethyl Ketones
  • Carrier Proteins
  • Caspase Inhibitors
  • Fullerenes
  • Inflammasomes
  • Interleukin-1beta
  • NLR Family, Pyrin Domain-Containing 3 Protein
  • NLRP3 protein, human
  • Nanotubes, Carbon
  • RNA, Small Interfering
  • benzyloxycarbonyltyrosyl-valyl-alanyl-aspartic acid fluoromethyl ketone
  • Caspase 1