Neither azeotropic drying, nor base nor other additives: a minimalist approach to (18)F-labeling

Org Biomol Chem. 2014 Oct 28;12(40):8094-9. doi: 10.1039/c4ob01336k.

Abstract

A novel, efficient, time-saving and reliable radiolabeling procedure via nucleophilic substitution with [(18)F]fluoride is described. Different radiolabeled aliphatic and aromatic compounds were prepared in high radiochemical yields simply by heating of quaternary anilinium, diaryliodonium and triarylsulfonium [(18)F]fluorides in suitable solvents. The latter were obtained via direct elution of (18)F(-) from an anion exchange resin with alcoholic solutions of onium precursors. Neither azeotropic evaporation of water, nor a base, nor any other additives like cryptands or crown ethers were necessary. Due to its simplicity this method should be highly suitable for automated radiosyntheses, especially in microfluidic devices.

MeSH terms

  • Aniline Compounds / chemistry*
  • Fluorine Radioisotopes / chemistry*
  • Isotope Labeling
  • Microfluidic Analytical Techniques
  • Onium Compounds / chemistry*
  • Sulfonium Compounds / chemistry*

Substances

  • Aniline Compounds
  • Fluorine Radioisotopes
  • Onium Compounds
  • Sulfonium Compounds