Effect of amines as activators on the alcohol-oxidizing activity of pyrroloquinoline quinone-dependent quinoprotein alcohol dehydrogenase

Biosci Biotechnol Biochem. 2014;78(7):1195-8. doi: 10.1080/09168451.2014.917265. Epub 2014 May 28.

Abstract

Pyrroloquinoline quinone-dependent quinoprotein alcohol dehydrogenases (PQQ-ADH) require ammonia or primary amines as activators in in vitro assays with artificial electron acceptors. We found that PQQ-ADH from Pseudomonas putida KT2440 (PpADH) was activated by various primary amines, di-methylamine, and tri-methylamine. The alcohol oxidation activity of PpADH was strongly enhanced and the affinity for substrates was also improved by pentylamine as an activator.

Keywords: alcohol dehydrogenase; alkyl amine; enzyme activator; pyrroloquinoline quinone; quinoprotein.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alcohol Oxidoreductases / metabolism*
  • Alcohols / metabolism*
  • Amines / pharmacology*
  • Dose-Response Relationship, Drug
  • Enzyme Activation / drug effects
  • Oxidation-Reduction / drug effects
  • PQQ Cofactor / metabolism*
  • Pseudomonas putida / enzymology

Substances

  • Alcohols
  • Amines
  • PQQ Cofactor
  • Alcohol Oxidoreductases
  • alcohol dehydrogenase (acceptor)