One-nanometer-precision control of Al(2)O(3) nanoshells through a solution-based synthesis route

Angew Chem Int Ed Engl. 2014 Nov 17;53(47):12776-80. doi: 10.1002/anie.201406856. Epub 2014 Oct 21.

Abstract

Forming uniform metal oxide nanocoatings is a well-known challenge in the construction of core-shell type nanomaterials. Herein, by using buffer solution as a specific reaction medium, we demonstrate the possibility to grow thin nanoshells of metal oxides, typically Al2 O3 , on different kinds of core materials, forming a uniform surface-coating layer with thicknesses achieving one nanometer precision. The application of this methodology for the surface modification of LiCoO2 shows that a thin nanoshell of Al2 O3 can be readily tuned on the surface for an optimized battery performance.

Keywords: Al2O3 coating; core-shell structure; layer thickness; lithium-ion batteries.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Aluminum Oxide / chemical synthesis*
  • Aluminum Oxide / chemistry*
  • Nanostructures / chemistry*
  • Particle Size
  • Solutions
  • Surface Properties

Substances

  • Solutions
  • Aluminum Oxide