Corynanthean, eburnan, secoleuconoxine, and pauciflorine alkaloids from Kopsia pauciflora

Phytochemistry. 2014 Dec:108:234-42. doi: 10.1016/j.phytochem.2014.09.014. Epub 2014 Oct 17.

Abstract

Eleven indole alkaloids, comprising four corynanthean, two eburnane, one aspidofractinine, one secoleuconoxine, one andranginine, and two pauciflorine type alkaloids were isolated from the stem-bark and leaf extracts of Kopsia pauciflora. Their structures were determined using NMR and MS analyses. The catharinensine type alkaloid kopsirensine B and the secoleuconoxine alkaloid arboloscine A showed moderate to weak activity in reversing MDR in vincristine-resistant KB cells. The alkaloid content was markedly different compared to that of a sample from Malaysian Borneo.

Keywords: Apocynaceae; Indole alkaloids; Kopsia pauciflora; NMR; Reversal of multidrug-resistance.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antineoplastic Agents, Phytogenic / chemistry
  • Antineoplastic Agents, Phytogenic / isolation & purification*
  • Antineoplastic Agents, Phytogenic / pharmacology
  • Apocynaceae / chemistry*
  • Drug Resistance, Multiple / drug effects
  • Drug Resistance, Neoplasm / drug effects
  • Drug Screening Assays, Antitumor
  • Humans
  • Indole Alkaloids / chemistry
  • Indole Alkaloids / isolation & purification*
  • Indole Alkaloids / pharmacology
  • KB Cells
  • Lactams
  • Malaysia
  • Molecular Structure
  • Nuclear Magnetic Resonance, Biomolecular
  • Plant Bark / chemistry
  • Plant Leaves / chemistry
  • Vincristine / pharmacology

Substances

  • Antineoplastic Agents, Phytogenic
  • Indole Alkaloids
  • Lactams
  • andranginine
  • aspidofractinine
  • corynanthean
  • eburnan
  • pauciflorine A
  • pauciflorine B
  • secoleuconoxine
  • Vincristine