L-1416, a novel MDR reversing agent with possible reduced calcium antagonism

Pharmacol Rep. 2014 Dec;66(6):1140-7. doi: 10.1016/j.pharep.2014.07.003. Epub 2014 Aug 2.

Abstract

Background: Multidrug efflux transporter P-glycoprotein (P-gp) is highly expressed on membrane of tumor cells and supposed to be implicated in the resistance to tumor chemotherapy. However, currently none of P-gp inhibitors has been approved by Food and Drug Administration not only due to toxicity but also lack of efficacy in clinical trials.

Methods: To solve the problem, our lab synthesized a novel compound named 1416 [1-(2,6-dimethylphenoxy)-3,4-dimethoxyphenylethylamino) propane hydrochloride] with the hope of high P-gp inhibition and low side effects. Caco-2 cell monolayer and tumor bearing mice were used to evaluate the P-gp inhibition of 1416 in vitro and in vivo, respectively. One of its potential side effects, calcium antagonism was also evaluated.

Results: Results showed that 1416 showed a similar P-gp inhibition as verapamil in Caco-2 cell monolayer. No significant difference was observed in antitumor enhancement when the optical isomers of 1416 (D-1416 and L-1416) were co-administered with vinblastine. In calcium antagonism, L-1416 showed less calcium inhibition than both D-1416 and verapamil.

Conclusion: The novel compound 1416 could significantly increase the antitumor effects of cytotoxic drugs and one of its optical isomers, L-1416, might be more promising due to its potential low calcium antagonism.

Keywords: Calcium antagonism; L-1416; P-gp inhibitor; Tumor therapy.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • ATP Binding Cassette Transporter, Subfamily B, Member 1 / antagonists & inhibitors*
  • Animals
  • Antineoplastic Agents / pharmacology*
  • Caco-2 Cells
  • Calcium / metabolism*
  • Drug Resistance, Neoplasm
  • Humans
  • Mice
  • Phenethylamines / chemistry
  • Phenethylamines / pharmacology*
  • Phenethylamines / toxicity
  • Propylamines / chemistry
  • Propylamines / pharmacology*
  • Propylamines / toxicity
  • Stereoisomerism
  • Verapamil / pharmacology
  • Vinblastine / pharmacology

Substances

  • 1-(2,6-dimethylphenoxy)-3,4-dimethoxyphenylethylamino)propane
  • ATP Binding Cassette Transporter, Subfamily B, Member 1
  • Antineoplastic Agents
  • Phenethylamines
  • Propylamines
  • Vinblastine
  • Verapamil
  • Calcium