Characterization of semiquinone free radicals formed from stilbene catechol estrogens. An ESR spin stabilization and spin trapping study

J Biol Chem. 1989 Jul 5;264(19):11014-9.

Abstract

Electron spin resonance spectroscopy has been used to detect, characterize, and to infer structures of o-semiquinones derived from stilbene catechol estrogens. Radicals were generated enzymatically using tyrosinase and were detected as their Mg2+ complexes. It is suggested that initial hydroxylation of stilbene estrogen gives a catechol estrogen in situ; subsequent two-electron oxidation of the catechol to the quinone, followed by reverse disproportionation, leads to the formation of radicals. Consistent with this mechanism, o-phenylenediamine, a quinone trapping agent, inhibits formation of o-semiquinones. A competing mechanism of radical production involves autoxidation of the catechol. Hydroxyl radicals are shown to be produced in this system via a mechanism involving reduction of iron and copper complexes by stilbene catechols. Possible differences in the reactivity of stilbene ortho- and para-semiquinones are discussed.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Benzoquinones*
  • Cyclic N-Oxides
  • Dienestrol / analogs & derivatives
  • Dienestrol / metabolism
  • Diethylstilbestrol / analogs & derivatives
  • Diethylstilbestrol / metabolism
  • Electron Spin Resonance Spectroscopy*
  • Estrogens, Catechol / metabolism*
  • Free Radicals
  • Hexestrol / analogs & derivatives
  • Hexestrol / metabolism
  • Magnesium / metabolism
  • Molecular Structure
  • Monophenol Monooxygenase / metabolism
  • Oxidation-Reduction
  • Quinones*
  • Spin Labels
  • Stilbenes* / metabolism*

Substances

  • Benzoquinones
  • Cyclic N-Oxides
  • Estrogens, Catechol
  • Free Radicals
  • Quinones
  • Spin Labels
  • Stilbenes
  • Hexestrol
  • semiquinone radicals
  • 5,5-dimethyl-1-pyrroline-1-oxide
  • Diethylstilbestrol
  • Monophenol Monooxygenase
  • Magnesium
  • Dienestrol