Phainanoids A-F, a new class of potent immunosuppressive triterpenoids with an unprecedented carbon skeleton from Phyllanthus hainanensis

J Am Chem Soc. 2015 Jan 14;137(1):138-41. doi: 10.1021/ja511813g. Epub 2014 Dec 24.

Abstract

Phainanoids A-F (1-6), six highly modified triterpenoids with a new carbon skeleton by incorporating two unique motifs of a 4,5- and a 5,5-spirocyclic systems, were isolated from Phyllanthus hainanensis. Their structures with absolute configurations were determined by spectroscopic data, chemical methods, and X-ray crystallography. Compounds 1-6 exhibited exceptionally potent immunosuppressive activities in vitro against the proliferation of T and B lymphocytes. The most potent one, phainanoid F (6), showed activities against the proliferation of T cells with IC50 value of 2.04 ± 0.01 nM (positive control CsA = 14.21 ± 0.01 nM) and B cells with IC50 value of <1.60 ± 0.01 nM (CsA = 352.87 ± 0.01 nM), which is about 7 and 221 times as active as CsA, respectively. The structure-activity relationships of 1-6 are discussed.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • B-Lymphocytes / drug effects
  • Carbon / chemistry*
  • Cell Proliferation / drug effects
  • Cell Survival / drug effects
  • Concanavalin A / antagonists & inhibitors
  • Concanavalin A / pharmacology
  • Crystallography, X-Ray
  • Dose-Response Relationship, Drug
  • Immunosuppressive Agents / chemistry*
  • Immunosuppressive Agents / isolation & purification*
  • Immunosuppressive Agents / pharmacology
  • Lipopolysaccharides / antagonists & inhibitors
  • Lipopolysaccharides / pharmacology
  • Mice
  • Models, Molecular
  • Molecular Conformation
  • Phyllanthus / chemistry*
  • Stereoisomerism
  • Structure-Activity Relationship
  • T-Lymphocytes / drug effects
  • Triterpenes / chemistry*
  • Triterpenes / isolation & purification*
  • Triterpenes / pharmacology

Substances

  • Immunosuppressive Agents
  • Lipopolysaccharides
  • Triterpenes
  • Concanavalin A
  • Carbon