Selective recognition of Ni2+ ion based on fluorescence enhancement chemosensor

Spectrochim Acta A Mol Biomol Spectrosc. 2015 Apr 5:140:283-7. doi: 10.1016/j.saa.2014.12.042. Epub 2014 Dec 24.

Abstract

A new enhancing fluorescent chemosensor was introduced for selective and sensitive determination of nickel ions based on 2-(1-H-benzo[d]imidazol-2yl)-N-phenyl hydrazine carbothioamide (L). L has an intrinsic fluorescent emission which enhances in presence of nickel ions in CH3CN/H2O (70:30, v/v) solution. The fluorescence enhancement of L is attributed to a 1:1 complex formation between L and Ni2+ ion which has been used for selective detection of Ni2+ ion. At the optimum conditions, the fluorescence intensity of L at 352 nm enhances linearly by the concentration of nickel ion from 1.6×10(-5) to 1.6×10(-7) M and detection limit of 7.9×10(-8) M. The new fluorescent probe exhibited high selectivity to Ni2+ ion over the other common mono, di-and trivalent cations.

Keywords: Enhancement; Fluorescence; Nickel; Selective Ion Recognition; Sensor.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cations, Divalent / analysis
  • Fluorescence
  • Fluorescent Dyes / chemistry*
  • Limit of Detection
  • Nickel / analysis*
  • Phenylhydrazines / chemistry*
  • Spectrometry, Fluorescence / methods
  • Thioamides / chemistry*
  • Wastewater / analysis
  • Water / analysis

Substances

  • Cations, Divalent
  • Fluorescent Dyes
  • Phenylhydrazines
  • Thioamides
  • Waste Water
  • Water
  • Nickel